RRC ID 41405
Author Arima H, Kihara F, Hirayama F, Uekama K.
Title Enhancement of gene expression by polyamidoamine dendrimer conjugates with alpha-, beta-, and gamma-cyclodextrins.
Journal Bioconjug Chem
Abstract To improve the transfection efficiency of nonviral vector, we synthesized the starburst polyamidoamine dendrimer conjugates with alpha-, beta-, and gamma-cyclodextrins (CDE conjugates), expecting the synergistic effect of dendrimer and cyclodextrins (CyDs). The (1)H NMR spectroscopic data indicated that alpha-, beta-, and gamma-CyDs are covalently bound to dendrimer in a molar ratio of 1:1. The agarose gel electrophoretic studies revealed that CDE conjugates formed the complexes with plasmid DNA (pDNA) and protected the degradation of pDNA by DNase I in the same manner as dendrimer. CDE conjugates showed a potent luciferase gene expression, especially in the dendrimer conjugate with alpha-CyD (alpha-CDE conjugate) which provided the greatest transfection activity (approximately 100 times higher than those of dendrimer alone and of the physical mixture of dendrimer and alpha-CyD) in NIH3T3 and RAW264.7 cells. In addition, the gene transfer activity of alpha-CDE conjugate was superior to that of Lipofectin. The enhancing gene transfer effect of alpha-CDE conjugate may be attributable to not only increasing the cellular association, but also changing the intracellular trafficking of pDNA. These findings suggest that alpha-CDE conjugate could be a new preferable nonviral vector of pDNA.
Volume 12(4)
Pages 476-84
Published 2001-1-1
DOI 10.1021/bc000111n
PII bc000111n
PMID 11459450
MeSH 3T3 Cells / metabolism Animals Binding Sites / physiology Cyclodextrins / chemistry Cyclodextrins / pharmacology* DNA / chemistry DNA / metabolism* Deoxyribonuclease I / metabolism* Drug Synergism Gene Expression / drug effects* Gene Transfer Techniques Genetic Vectors / genetics Mice Microscopy, Confocal Phosphatidylethanolamines / pharmacology Plasmids / chemistry Polymers / pharmacology* Transfection
IF 4.031
Times Cited 198
WOS Category CHEMISTRY, ORGANIC BIOCHEMICAL RESEARCH METHODS CHEMISTRY, MULTIDISCIPLINARY BIOCHEMISTRY & MOLECULAR BIOLOGY
Altmetric score
オルトメトリクス指標項目
The most frequently cited source Patent(IFI CLAIMS)
Total number of mentions 11
Altmetric score changes over past 6months 0.0
Resource
Human and Animal Cells RAW 264(RCB0535)